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A polymer (CHS 2 ) n  and sulfate are formed in the γ-irradiation of deaerated aqueous carbon disulfide solutions. The G-values are 3.6 and 0.41, respectively. In the presence of N,O, G (polymer) is decreased while G(SO 4  - ) is increased. G(SO 4  - ) can be decreased by isopropanol. G(polymer) is increased by H +  ions and reaches a value of 5 below pH = 2. Formic acid, hydrogen sulfide and carbonate are formed in the hydrolysis of the polymer. Pyrolysis at first leads to a red oil consisting of oligomer (HCS 2 ) n  and finally to H 2 S, CS 2  plus a residue containing much carbon. The structure of the polymer is discussed.

zeitschrift für naturforschung b

Die γ-Radiolyse und Pulsradiolyse des Schwefelkohlenstoffs in wäßriger Lösung / The γ-Radiolysis and Pulse Radiolysis of Carbon Disulfide in Aqueous Solution