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A harmonic-vibration analysis for the vibrations of 1,3,5,7-cyclooctatetraene was performed. A suitable set of symmetry coordinates is specified, and the corresponding symmetry force constants for C 8 H 8  are given. The developed force fields were used to calculate mean amplitudes of vibration for C 8 H 8  and C 8 D 8 . Calculated perpendicular amplitude correction coefficients for the various interatomic distances are also reported.

IV. 1,3,5,7-Cyclooctatetraene: Mean Amplitudes of Vibration of Comparatively Large Molecules