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A local short-to-intermediate range order of liquid Al 80 Co 10 Ni 10 , Al 72.5 Co 14.5 Ni 13 , and Al 65 Co 17.5 Ni 17.5  alloys was examined by X-ray diffraction and the reverse Monte Carlo modelling. The comprehensive analysis of three-dimensional models of the liquid ternary alloys was performed by means of the Voronoi-Delaunay method. The existence of a prepeak on the S(Q) function of the liquid alloys is caused by medium range ordering of 3d-transition metal atoms in dense-packed polytetrahedral clusters at temperatures close to the liquidus. The non-crystalline clusters, represented by aggregates of pentagons that consist of good tetrahedra, and chemical short-range order lead to the formation of the medium range order in the liquid binary Al-Ni, Al-Co and ternary Al-Ni-Co alloys.

Short and Medium-Range Order in Liquid Ternary Al 80 Co 10 Ni 10 , Al 72.5 Co 14.5 Ni 13 , and Al 65 Co 17.5 Ni 17.5 Alloys