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The molar enthalpies of mixing (Δ mix H m ) of liquid PrCl 3 -LiCl and NdCl 3 -LiCl mixtures have been measured at 1044 K. For both systems these enthalpies are negative in the whole composition range, with a minimum at x PrCl3  and x NdCl3  ≈ 0.4. The results are compared with existing mixing enthalpy data on lanthanide chloride-alkali metal chloride systems and discussed in terms of complex formation in the melts.

Enthalpy of Mixing of the PrCl 3 -LiCl and NdCl 3 -LiCl Molten Salt Systems