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The rate of the degenerate isomerization of N-hexafluoroisopropylidene-N’,N’-dimethyl-ρ-phe-nylenediamine was measured by high-pressure  19 F NMR spectroscopy in a viscous hydrocar-bon, 2,4-dicyclohexyl-2-methylpentane. Pressure-induced retardations that cannot be rationalized within the framework of the transition state theory (TST) were observed, and it was concluded that the reaction was cast into the TST-invalid nonequilibrium conditions by high pressure.

Dynamic Solvent Effects in the Degenerate Isomerization of a Hexafluoroacetone Anil Studied by High-Pressure 19 F NMR