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By the sol-gel method, a polycrystal bulk of two-layered La 2-2x Ca 1+2x Mn 2 O 7  with x = 0.2 was successfully synthesized. A high sensitive low-field TMR was found at low temperature.

Tunneling Magnetoresistance in a Two-Layered La 2-2x Ca 1+2x Mn 2 O 7 Polycrystal