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Electric polarizabilities and hyperpolarizabilities were calculated from accurate self-consistent field wavefunctions for P 2 . The following values are reported, using the experimental bond length of 1.8934 Å: dipole polarizability α zz  = 69.83 and α xx  = 41.20 e 2  a 0  2  Eh -1  , second dipole hyperpolarizability γ zzzz  = 17 040, γ xxxx = 11 581 and γ xxzz  = 4724 e 4 a 0  4 E h  -3 , quadrupole polarizability, C zz „zz  = 276.14, C xz,xz  = 232.64 and C xx,xx  = 151.25 e 2  a 0  4 E h  -1  , dipole-octopole polarizability, E z,zzz , = 331.00 and E x,xxx  = -154.66 e 2  a 0  4 E h  -1  and for the dipole-dipole-quadrupole hyperpolarizability, B zz,zz  = - 2441, B xz,xz  = - 1442, B xx,zz  = 866 and B xx,xx  = - 1411 e 3 a 0  4 Eh -2 .

Linear and Non-linear Polarizabilities for P 2 (X 1 Σ g + )