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The electric field gradient at the fluorine site of several crystalline trifluorides was measured by means of the time differential perturbed angular distribution method. The hyperfine data (v Q  and η) are systematically analyzed by taking into account the structural parameters of the crystals; they are also compared to the results obtained by point charge calculations.

Systematic Investigation of MF 3 Crystalline Compounds (M = Al, Cr, Fe, Ga, In, Sc, Ti, and V) and Fe 1-x M x F 3 Mixed Series (M = Ga, Cr, V)