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The nuclear quadrupole coupling of [ 35 Cl, 35 Cl]- and [ 35 Cl,Cl]-sulfur dichloride was investigated using waveguide microwave Fourier transform (MWFT) spectroscopy. The analysis was performed with direct diagonalization of the Hamilton matrix. Due to some measured transitions with near degeneracy it was possible to determine the off diagonal elements χ ab  of the quadrupole coupling tensor with high accuracy.

Quadrupole Hyperfine Structure in the Rotational Spectra of Sulfur Dichloride