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The  14 N hyperfine multiplets of low-7 rotational transitions of the E and Z isomers of HN = CH - C ≡ N, produced by flash pyrolysis from (CH 3 ) 2 N -C ≡ N as precursor, were observed and analysed. The quadrupole coupling constants determined are  (c -axis perpendicular to the molecular plane):

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The  14 N Nuclear Quadrupole Coupling in E- and Z-C-Cyanomethanimine; its Prediction from Restricted Hartree-Fock Wave Functions and its Experimental Determination by High Resolution Microwave Spectroscopy