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The zero field  14 N-hfs-multiplets and the high-field Zeeman-hfs-multiplets of low-J rotational transitions of the title compounds were observed in a flash pyrolysis setup under high-resolution conditions. From the zero-field hfs patterns the  14 N spin-rotation coupling constants and the  14 N nuclear quadrupole coupling constants were obtained. From the high-field Zeeman-hfs-multiplets, the diagonal elements of the molecular g-tensor and the anisotropies in the diagonal elements of the molecular magnetic susceptibility tensor were determined and were used to derive the diagonal elements of the molecular electric quadrupole moment tensor. INDO calculations and restricted Hartree-Fock self consistent field calculations with a basis of TZVP quality were carried out at the experimental structures and critically compared to the experimental results

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The Rotational Zeeman Effect of Imines II. Cis- and Trans-Ethanimine and Trans-Syn- and Trans-Anti-Propenimine, their g-Tensors, Magnetic Susceptibility Anisotropics, Molecular Electric Quadrupole Moments,  14 N Nuclear Quadrupole Coupling Constants, and  14 N Spin-Rotation Coupling Constants; a Microwave Spectroscopic Study Combined with Quantum Chemical Calculations