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Information from rotational spectroscopy has been utilised for the interpretation of experimental results from laser/microwave double resonance (LMDR) experiments on furazan. The band origins v 0  for the fundamental vibrations v 12  and v 5  have been deduced from these experiments as v 0  12  = 952.611 (2) cm  -1  and = 1005.353(2] cm -1

Vibrational Band Origins of the Fundamentals v 12 and v 5 of Furazan from Laser/Microwave Double Resonance