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X-ray scattering measurements have been done on aqueous MgCl 2 -KCl and MgCl 2  CsCl solutions saturated with their double salts of MgCl 2 • KCl • 6 H 2 O and MgCl 2  • KCl • 6 H 2 O respectively, at 293 K. The Mg 2+  ion was found to be coordinated with six water molecules at an Mg-O distance of 209 and 208 pm, respectively, whereas K +  and Cs +  ions were surrounded by both water molecules and chloride ions in the first coordination sphere. The interatomic distance between the alkali cation and the chloride ion was 320 pm and 339 pm for K +  and Cs +  , respectively, and the coordination numbers of K +  and Cs +  with respect to CP were 2.4 and 2.0, respectively. The alkali metal H20 distance and the hydration number of the cation were 277 pm and 3.7, respectively, for K +  and 315 pm and 4.7, respectively, for Cs +  . The structures of the solutions are discussed in connection with the nucleation processes of the salts from the aqueous solutions

X-Ray Diffraction Studies on Ternary MgCl 2 -KCI-H 2 O and MgCI 2 -CsCl-H 2 O Solutions Saturated with the Corresponding Double Salts