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The rotational spectra of pyridine-N-oxide and x-picoline-N-oxide ( = 2-methvlpyridine-N-oxide) have been observed by means of pulsed microwave spectroscopy. For both molecules, the  14 N quadrupole coupling constants have been obtained. For α-picoline-N-oxide. in addition the parameters of the internal rotation motion and the centrifugal distortion constants have been determined.

High Resolution Microwave Spectra of Pyridine-N-oxideanda-Picoline-N-oxide