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The  14 N hyperfine structure in the rotational spectra of cyclopropylamine and cyclopropyl cyanide has been reinvestigated by microwave Fourier transform spectroscopy. The observed quadrupole coupling constants in units of MHz are: X aa  = 2.3338(18), X bb  = 1.7874(20), X cc  = −4.1209(20) for cyclopropylamine and X aa  = −3.4536(35), X bb = 1.7468(51), X cc = 1.7068(51) for cyclopropyl cyanide.

14 N Quadrupole Coupling in the Rotational Spectra of Cyclopropylamine and Cyclopropyl Cyanide