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A nonlinear enzyme reaction in a chemical gradient with an artificial feed-back loop is modified by the application of a constant temperature gradient leading to laminar convective motion of the fluid at an electrode. The complete system is shown to undergo a bifurcation into a limit cycle as a function of the applied temperature gradient. The effect of other parameters on the oscillation is described. More complicated types of behavior are expected in parameter space.

A New Model System for the Study of Complex Dynamical Enzyme Reactions. II. Oscillations in a Reaction-Diffusion-Convection System