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The microwave and millimeterwave spectrum of  15 N-fluoracetonitrile(CH 2 FC 15 N) in the ground vibrational state are investigated in the region between 8 and 150 GHz. The measured transitions are fitted to a Hamiltonian with three rotational constants, five quartic and seven sextic centrifugal distortion constants in the symmetric top limit of van Eijck-Typke and in the s-reduction of Watson. The rotational constants are used to improve the calculated r 0  -restructure of the fluoracetonitrile molecule.

Microwave and Millimeterwave Spectrum of Monofluoracetonitrile- 15 N (CH 2 FC 15 N). A Contribution to Molecular Structure