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The quadrupole and spin rotation coupling constants are determined by analysis of the J = 0 - 1 and J = 1 - 2 transitions o f OC 33 S and  17 OCS in natural abundance. The data are compared with those obtained from molecular beam electric resonance and very recent pulsed beam microwave Fourier transform spectroscopy.

Determination of Quadrupole and Spin-Rotation Coupling in the Rotational Spectrum of Carbonylsulfide- 33 S and - 17 O