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Two models for a plane interface between a free electron metal and a concentrated solution of a surface inactive electrolyte are treated fully self-consistently, taking into account both the polarizability of the metallic electron cloud and the reorientation of solvent molecules. The interfacial capacity is calculated as a function of the electrode charge, and its dependence on various system parameters is investigated. Some conclusions on the structure of the interface are drawn from a comparison between our results and experimentally observed trends.

Self-Consistent Density Functional Approach to a Metal/Electrolyte Solution Interface