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With use of a Fourier transform microwave spectrometer in the range of 4 GHz to 18 GHz, the pressure dependence of collisional coherence dephasing times T 2  at room temperature has been determined for (a) the transition J = 0 → J =1 of OCS,  18 OCS, and OC 34 S, (b) nine transitions of SO 2  in ground state having 13 ≦ J ≦ 59, and (c) eight transitions of SO 2  having 12 ≦ 7 ≦ 55 in the first excited bending vibrational state, where J is the rotational quantum number of the lower state.

A Contribution to the Investigation of T 2 -Relaxation: Rotational Transitions of OCS and SO 2