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Rotational spectra of dimethyl selenide in torsional and vibrational excited states were measured by Stark-and MWMW double resonance spectroscopy. The spectra could be assigned partially and evaluated for internal rotation parameters. The limitation of the rigid top-rigid frame Hamiltonian became obvious.

A Contribution to the Analysis of the Rotational Spectra of Dimethyl Selenide in Torsional Excited States