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Phenyl-t-butylketone (pivalophenone) was irradiated in mixtures of benzene and 2-propanol with 25 ns flashes of 347.1 nm light. Triplet lifetimes were measured by monitoring the decay of the T-T-absorption. 2-propanol exerts a significant stabilizing influence upon the triplet lifetime and lowers the triplet reactivity probably due to a n, π* → π, π* inversion of the lowest triplet state.

Solvent Dependence of the Triplet Reactivity of Pivalophenone as Evidenced by Laser Flash Photolysis