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13 C/ 12 C reduced isotopic partition function ratios for the three singly  13 C substituted cyanoacetylenes are calculated and are used to evaluate the thermodynamic equilibrium constants among these species. A perturbation theory method is employed to dissect both the partition function ratios and also the equilibrium constants in order to gain a better understanding of isotope effects.

Dissection of 13 C/ 12 C Isotope Effects on the Cyanoacetylene Partition Function