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The microwave rotational spectrum of the most abundant species of 3-Cyanothiophene was investigated for the ground vibrational state. Rotational constants and centrifugal distortion constants are given. The electric dipole moment components μ a  and μ b  and the  14 N-quadrupole coupling constant X  +  = X  bb  + X  cc  were determined from the Stark-effect splittings and hfs-splittings respectively. The experimental results are compared to CNDO/2 calculations and are discussed with reference to ring distortion.

Rotational Spectrum , Electric Dipole Moment, Quadrupole Coupling , and Partial r 0 - Structure of 3 -Cyanothiophene