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The magnetic susceptibilities of some transition metal (II) complexes with 1,2,4-triazole (trz) have been measured in the range 2-300 K. Ni (trz) 2  (NO 3 ) 2  (H 2 O)  8/3 , Ni (trz) 2  SO 4  (H 2 O) 5  and α-Ni (trz) 2  (NCS) 2  are found to be linear antiferromagnetic trimers. For β- Ni (trz) 2  (NCS) 2  and similar compounds with Mn (II), Fe (II), Co (II) and Cu(II), totally different magnetic properties were observed, suggesting the presence of two-dimensional networks of metal ions bridged by 1,2,4-triazole molecules. For Co (trz)  2  (NCS)  2  this was confirmed by X-ray single crystal diffraction.

Magnetic Susceptibility and Structure of Some Transition Metal (II) Complexes with 1,2,4-Triazole