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Fall-off curves for the reaction ClO+NO 2 (+N 2 )→ClONO 2 (+N 2 ) at 300 and 220 K have been calculated from Kassel integrals by use of a theoretically derived high pressure limit and the experimentally determined low pressure limit as reference points. The reaction is found to deviate considerably from the low pressure limit at pressures larger than 10 Torr. Effective rate constants for the use in atmospheric models of chlorine nitrate formation are derived.

Fall-Off Curves for the Reaction ClO + NO 2 ( + N 2 ) ClONO 2 (+N 2 )