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A single component hard sphere description molten halides and nitrates, applied to self-diffusion and viscosity data, has led to a hard sphere size which for a given cation depends linearly upon the anionic radius. This correlation has been used to predict viscosity coefficients of fused alkali fluorides and to estimate the effective size of the NO 3  -  -anion in molten nitrates. The Stokes-Einstein relationship between η and D̅ is satisfied, where D̅= (D +  +D - )/2, and this relationship in combination with the observed linear dependence of T½/η] and D̅/T½ on the molar volume can in principle be used as a criterion for data selection.

Hard-sphere Results from Experimental Transport Behaviour of Molten Salts and Structural Properties