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Unstabilized N 2 (B 3 II g , ν = 13) quasi-molecules were analysed by excitation with a tunable dye-laser into the N 2 (C 3 II u ) state and observation of the following fluorescence to N 2 (B 3 II g , ν) levels. The quasi-molecules are in equilibrium with the free nitrogen atoms. The detection limit of this technique is 10 5  molecules/cm 3 . By the same method, a rotational analysis of molecules stabilized into (B 3 II g , ν ≦ 12) levels by three-body recombination processes was achieved with a resolution better than that reached by emission spectroscopy of the Lewis-Rayleigh afterglow

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Laserspektroskopische Untersuchungen an nicht-stabilisierten N 2 (B 3 II g , ν; = 13)-Molekülen / Laser Spectroscopic Studies on Non-stabilized N 2 (B 3 II g , ν; = 13) molecules