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Short-range interactions of Electrolyte Solutions Short range interaction potentials between ions are approximated by a step function with a hard core. Then from general statistical-mechanical formulas the first correction to the limiting law of the free excess energy F* (S (2)  -term of the cluster theory) is computed for low concentrations, i.e. small plasm parameter μ=e 2  x/D 0  kT ⪡ -. Fitting to a Lennard-Jones potential for symmetrical electrolytes results in values for F*, the osmotic pressure and the osmotic coefficient. Numerical fitting to experimental results of Lange for the osmotic coefficient gives information concerning the contact distance a and attraction parameter E for some water-tetraalkylhalogenide-systems.

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Berechnung der freien Exzeßenergie und des osmotischen Koeffizienten zur Gewinnung von Potential-Parametern kurzreichender Wechselwirkungen bei Elektrolytlösungen