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The pure rotational spectrum of vinyl isocyanide in the ground vibrational state has been as-signed in the frequency region from 8 GHz to 180 GHz. The measured absorption lines encompass 157 a-type transitions from the  q R K  ,  q Q 1 ,  q Q 2,  q Q 3 ,  q Q 4  and  q Q 5  branches and 48 b-type transitions from the  r P 0  ,  r P 1 ,  r P 2 ,  r P 3  ,  r P 4  ,  r P 5 ,  r Q 0  , and  r Q 1  branches for values of J up to 54. The rotational constants have been refined and all quartic and sextic centrifugal distortion constants have been determined using Watson's reduced Hamiltonian. No quadrupole hyperfine splitting was observed.

Ground State Centrifugal Distortion Constants of Vinyl Isocyanide, CH 2 -CH-NC, from the Microwave and Millimeter Wave Rotational Spectra