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Vapour pressures and vapour compositions of the liquid system water + acetic acid have been measured at 25 °C, 30 °C, 35 °C, 40 °C, and 45 °C in the whole range of compositions. The dimerization of acetic acid in the vapour being taken into account, the molar excess Gibbs function Ḡ E  is derived from the measurements. Earlier measurements of the molar excess enthalpy H E  are combined with the  - G E  values to give the molar excess entropy SE. The “symmetry rule” (Haase, 1951) concerning the composition dependence of Ḡ E ,  - H E , and S̄ E  has been confirmed.

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Verdampfungsgleichgewicht und thermodynamisehe Funktionen des flüssigen Systems Wasser + Essigsäure / Vapour-Liquid. Equilibrium and Thermodynamic Functions of the Liquid System Water + Acetic Acid