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The reactions producing vibrationally excited CO in the continuous wave CS 2  - O 2  chemical laser are considered. Fundamental and overtone transitions were observed in the systems CS 2  + O 2 , CS 2  + N 2 O, O 2  + CS and it is concluded that the two reactions O + CS → CO+S and O 2  + CS → CO + SO are the reactions in which vibrationally excited CO are produced. The second reaction appears to be responsible for overtone laser action at low buffer gas partial pressures and low discharge currents.

Investigations on the CS 2 —O 2 Chemical Laser