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The decompositions of doubly-charged ions given by a number of C 3  -C 8  aliphatic and alicyclic hydrocarbons have been investigated in a double-focusing mass spectrometer. Many processes were found in which high kinetic energy CH 3  +  and C 2 H 3  +  ions are formed. Doubly-charged ions fragment by more than one route and in many cases, high kinetic energy fragment ions are formed in at least two different ways. Metastable transitions common to several compounds were observed, the intensities rising as the degree of unsaturation increased.

Kinetic Energy Release and Metastable Transitions II. The Decomposition of Doubly-Charged Ions of Aliphatic and Alicyclic Hydrocarbons