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Several authors have observed the dissociation of a doubly charged CO 2  +  ion into CO +  and O + . There exist, however, discrepancies with respect to the transition energy (total translational energy). Therefore, the initial energy of O +  and CO +  ions formed by electron impact in CO 2  has been reinvestigated by the deflection method. Assuming dissociation into two fragments only, the transition energy can be calculated. In the initial energy distribution function of both ions a well pronounced satellite peak corresponding to the same transition energy of 5.5 eV is observed. This is interpreted as being due to the dissociation of a doubly charged CO 2  +  ion into two singly charged ions. The analogous dissociation of a metastable CO 2  +  ion is responsible for broad peaks at mass numbers 11.6 and 35.6 in the CO 2  mass spectrum. From the peak width a transition energy between 5 and 6 eV is calculated, indicating that the same excited state of CO 2  +  may be involved in both decomposition reactions

Die kinetische Energie ionisierter Molekülfragmente: V. Über einen ladungstrennenden Prozeß im CO 2 -Massenspektrum