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Indium selenide (InSe) film, an emerging two-dimensional chalcogenide semiconductor, has recently attracted growing interests in optoelectronics. However, its nonlinear characteristics and application potentials in mid-infrared (IR) region remain open, which is a very attractive but undeveloped spectral region currently. In this work, it is demonstrated that InSe film possesses excellent nonlinear absorption properties in 3- to 4-μm band. Saturable absorption measurements of InSe film at 2.8 and 3.5 μm show very low saturation energy fluences and moderate modulation depths. Pump–probe measurements at 3 and 4 μm indicate that InSe film has ultrafast responses in mid-IR region. Furthermore, the application of InSe film in mid-IR pulsed laser is demonstrated, and stable Q-switching operation of fiber laser at 2.8 μm is realized. These results show that InSe film is a promising saturable absorber for mid-IR pulsed laser.

Indium selenide film: a promising saturable absorber in 3- to 4-μm band for mid-infrared pulsed laser