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Under 254 nm irradiation cis-[Pt(C 6 H 5 CN) 2 Cl 2 ] is converted to H 2 PtCl 6 . Absorption of light by both the metal complex and the solvent contribute to the first step of this process, suggested to form HPt(C 6 H 5 CN) Cl 3 . A linear dependence of the reaction rate on light intensity appears to rule out chlorination by trichloromethyl radicals. However, at higher light intensities a higher order dependence on intensity develops, and under 313 nm irradiation is dominant, and a reaction between trichloromethyl radical and the excited state complex is proposed to account for this.

Kinetics of the Photosubstitution of ds-Bis(benzonitrile)dichloroplatinum(II) in Chloroform