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The vortex cavitation technology shows a great development potential for antibiotic wastewater treatment. We have designed a novel swirling vortex cavitator for tetracycline degradation in aqueous solution. By Computational Fluid Dynamics (CFD) simulation using ANSYS CFX flow field calculation software, it was found that the vortex cavitator could form a low-pressure area far lower than the saturated vapor pressure at experimental temperature, resulting in generation of obvious vortex cavitation effect, which also proved by the concentration of hydroxyl radical of 4.58 μmol/L measured by methylene blue method. Moreover, the tetracycline degradation process may be mainly caused by the oxidation of hydroxyl radicals. The batch experiments results showed when the degradation time was 30 min, the vortex cavitator had a good degradation ability of tetracycline in pH range of 5.0–9.0. The degradation efficiency of 2.0 mg/L tetracycline solution was 76.45% within 50 min at pH 7.0. The possible intermediate products of tetracycline were determined by HPLC-MS Spectrometry. A series of reactions including hydroxylation, decarbonylation and C–N bond cleavage, ring-opening, and removing two methyl groups in the carbon atom ring, occur during the degradation.

CFD simulation of a swirling vortex cavitator and its degradation performance and pathway of tetracycline in aqueous solution