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Autothermal reforming of CH 4  in a membrane catalytic microreactor for the production of hydrogen at different temperatures over supported Ni catalysts has been studied. A three-dimensional mathematical model was developed using a computational fluid dynamics (CFD) technique. The effect of using different membranes on the performance of the micro-reactor was analysed. The amounts of hydrogen produced and separated in each case, under the same operating conditions, were compared. It was proven that using the porous membrane (Ni–Al 2 O 3 ) could be an economic solution for the production and separation of hydrogen in membrane reactors.

Modelling of the Membrane Permeability Effect on the H 2 Production Using CFD Method