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The synthesis and characterization of  N -methacryloyl- L -tyrosine methyl ester (3a) and ethyl ester ( 3b ), and their acetyl derivatives  O -acetyl- N -methacryloyl-  L -tyrosine methyl ester ( 4a ) and ethyl ester ( 4b ) are described. Monomers  3  and  4  were complexed with RAMEB (randomly methylated  ß -cyclodextrin) yielding water soluble host-guest complexes  5a - d . The radical polymerization of monomers  3  and  4  was investigated in the presence as well as in the absence of RAMEB in aqueous medium at room temperature and also at 60°C. It is shown that the polymerization tendency of complexes  5a - d  at room temperature is lower, leading to polymers of higher molecular weight, compared to the free monomers  3  and  4 . Furthermore, the polymerization of monomers  3  and  4  was carried out in homogenous organic solution using 2,2’-azoisobutyronitrile as initiator, and the results are discussed.

e-polymers

Cyclodextrins in polymer synthesis: Dimethyl-β-cyclodextrin as thermosensitive retardant for the radical polymerization of N-methacryloyl-L-tyrosine derivatives in water