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We investigated molecular arrangement of organo-mod ified aluminosilicate with high surface coverage in Langmuir-Blodgett (LB) films by p erforming out-of-plane and in-plane X-ray diffraction (XRD) measurements. In addition, the surface morphology of mixed monolayers of organo-modified aluminosilicate and sev eral biodegradable polymers [e.g poly(L-lactide), PLLA] was also characterized by ato mic force microscopy (AFM).The in-plane XRD results of multilayers of organo-modif ied aluminosilicate formed by the LB method indicate the formation of a two-dimensional la ttice of hydrocarbons on the aluminosilicate surface. These hydrocarbons of organ o-modified reagents packed hexagonal in films. Based on our experimental findings, the LB t echnique enabled the formation of a densely packed organo-modified aluminosilicate mono layer at the water surface. Furthermore, for mixed monolayer systems comparising a n organo-modified clay with high surface coverage and biodegradable polymers, a misci ble surface was observed by AFM on a mesoscopic scales, whereas those with low surface co verage formed phase-separated structures.

Molecular Arrangement of Organo-modified Aluminosilicate in Langmuir-Blodgett Films and Mixed Monolayer Behavior with Biodegradable Polymers