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Manipulating polarization entanglement of paired photons is always of great interest for understanding the quantum nature of photons and exploring their applications in quantum information processing and quantum communication. Narrowband biphotons with polarization entanglement are especially important for a quantum network based on efficient photon–atom interactions. In most demonstrated cases, the polarization-entangled states are manipulated through the birefringent effect. In this Letter, we produce narrowband polarization-entangled biphotons from spontaneous four-wave mixing in cold atoms and demonstrate a new method to tune the phase of the polarization entanglement by varying the frequency of one of the classical driving lasers. This is achieved through two-photon interference with a path-exchange symmetry. Our result represents a precision control of polarization entanglement from the frequency domain, and may have promising applications in quantum information and precision measurement.

Frequency-induced phase-tunable polarization-entangled narrowband biphotons