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Cu2O is an interesting semiconductor with extraordinary high exciton binding energy, however exhibiting weak room temperature excitonic luminescence. The issue was addressed in literature emphasizing a detrimental role of native point defects responsible for optical quenching. Resolving the problem, we propose a method to manipulate the Cu and O vacancies contents opening a gateway for optoelectronic applications of Cu2O. Specifically, applying oxygen lean conditions, we observe a remarkable suppression of VCu enabling strong room temperature exciton luminescence, while manipulating with VO reveals no impact on the signal. As a result, the excitonic signature was interpreted in terms of phonon assisted transitions.

Engineering of optically defect free Cu_2O enabling exciton luminescence at room temperature