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We show that coherent anti-Stokes Raman lineshapes do not follow knownspectral profiles if the time asymmetry of realistic laser pulses is taken intoaccount. Examples are given for nanosecond and picosecond laser pulses commonlyemployed in frequency-resolved coherent anti-Stokes Raman scattering. Moreremarkably, the analysis suggests an effect of line narrowing in comparison tothe customary approach, based primarily on the Voigt lineshape.

Sensitivity of coherent anti-Stokes Raman lineshape to time asymmetry of laser pulses