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The recent measurement of negative higher-order Kerr effect (HOKE) terms ingases has given rise to a controversial debate, fed by its impact on shortlaser pulse propagation. By comparing the experimentally measured yield of thethird and fifth harmonics, with both an analytical and a full comprehensivenumerical propagation model, we confirm the absolute and relative values of thereported HOKE indices.

From higher-order Kerr nonlinearities to quantitative modeling of 3rd and 5th harmonic generation in argon