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We propose the extension of existing molecular modulation techniques for continuous-wave optical modulation to Raman-active microresonators. Intense pump and Stokes modes inside a microresonator prepare a high coherence of the Raman transition between two ro-vibrational states. With the coherence prepared, any laser in the optical region can be coupled to the microresonator and be modulated. We perform numerical simulations which predict that these "microresonator-based molecular modulators" could have modulation efficiencies on the order of 1% at 10 THz-scale frequencies for any optical wavelength.

Prospects for continuous-wave molecular modulation in Raman-active microresonators