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We use shaped near-infrared (NIR) pulses to control the generation ofcoherent broadband ultraviolet (UV) radiation in an atomic resonance-mediated(2+1) three-photon excitation. Experimental and theoretical results arepresented for phase controlling the total emitted UV yield in atomic sodium(Na). Based on our confirmed understanding, we present a new simple scheme forproducing shaped femtosecond pulses in the UV/VUV spectral range using thecontrol over atomic resonance-mediated generation of third (or higher order)harmonic.

NIR Femtosecond Control of Resonance-Mediated Generation of Coherent Broadband UV Emission