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The molecular and electronic structure of mononu- clear,dinuclear,polyuclear complexes and clusters of rare earths are discussed systematically,by an extended INDO me- thod made applicable to treat 4f-compounds,with respect to the nature of chemical bonding and factors influencing the coordination number and structural types of lanthanide com- plexes and organometallics.Some recent investigations in our laboratory on the synthesis,molecular and electronic struc- ture of some novel peroxy-bridging tetranuclear lanthanide complexes will also be discussed.

Coordination chemistry of rare earths: syntheses, structure, spectroscopy and chemical bonding