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The solubility of CO2 in pure water was investigated at high-pressure conditions, from 7 to 12 MPa, and at temperatures between 2.5-20°C. CO2 clathrate hydrate film formed at temperatures below approximately 10°C. The CO2 solubility was estimated by expanding the dissolved gas. The solubility decreased with decreasing temperature and with decreasing pressure, although some researchers reported it decreased with increasing pressure at 7°C, in the presence of the hydrate. Many other researchers reported that the pressure conditions did not affect the solubility in the presence of the hydrate. Although this seemed to be mostly correct, we did confirm a small difference of the solubility at pressures ranging 7-12 MPa.

The Effect on the CO2 Solubility into Water (Measurement of the CO2 Solubility by a Gas Expansion Method)