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Fourier transform IR absorption spectra of single crystals of the (ET)(2)C-60 complex grown from the CS2 solution as well as its components: C-60 and ET, also grown from CS2 solution, are presented and discussed. It is shown that the rotation of C-60 is strongly hindered and ET molecules are bent in the crystal structure of the complex. The arguments for the domination of the van der Waals interactions are given.

Infrared Absorption in Single Crystals of (ET)2C60Grown from CS2Solution

Infrared Absorption in Single Crystals of (ET)₂C₆₀Grown from CS₂Solution