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Magnetic and electronic properties of NdPd2Al3 have been nicely described with the Nd 3+ ions within the crystaleld theory revealing that all Nd atoms equally contribute to the temperature dependence of the paramagnetic susceptibility and of the heat capacity with the λ-peak. We consistently described paramagnetic and magnetically-ordered state. The ne electronic structure of the Nd ion nicely correlates with the electronic structure of the U ion in UPd2Al3 giving strong evidence for the trivalent uranium state in the isostructural heavy-fermion superconductor UPd2Al3.

Crystal-Field Interactions in RPd_2Al_3 Intermetallics (R = Pr, Nd, Sm, and U)